Research Interests
My current research interests cover a wide range of topics, some of which are relatively basic, such as Direct Methods, Surface Structures, and Density Functional Theory
and Flexoelectricity, while other, such as Hip Replacements, Catalysis, Corrosion and Tribology, have a stronger eye on applications; see the links below the Research tab above for
more details. Different from many research groups, we try more to focus on the science than any specific set of tools or techniques, an old-fashioned generalist approach. Much of the
fundamental work involves combining cutting-edge variants of electron microscopy in a unique combination of an electron microscope and surface science
system so we can combine more standard surface science probes, such as XPS or Auger, and chambers where samples are grown, all within one unique UHV system. Current projects include:
Flexoelectricity and Triboelectricity
A recent interest in flexoelectricity, and from this triboelectricity. Where does charge come from? We have been able to combine expertise in tribology to explain why charging
occurs in ways that were mysterious before. Key is the contribution of bending to the potential between materials which drives the charge transfer.
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Band Bending and Ratcheting Explain Triboelectricity in a Flexoelectric Contact Diode
K. P. Olson, C. A. Mizzi, and L. D. Marks
Nano Lett. 22 (2022) 3914-3921
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When Flexoelectricity Drives Triboelectricity
C. A. Mizzi and L. D. Marks
Nano Lett. 22 (2022) 3939-3945
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The role of surfaces in flexoelectricity
C. A. Mizzi and L. D. Marks
J. Appl. Phys. 129 (2021) 224102
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Does Flexoelectricity Drive Triboelectricity?
C. A. Mizzi*, A. Y. W. Lin*, and L. D. Marks (*equal contribution)
Phys. Rev. Lett. 123 (2019) 116103
Oxide Surfaces
At the current moment it is very hard to predict the structure of oxide surfaces; this is an important problem because these are very important in a large number of
different areas, ranging from catalysis through new types of oxide devices to corrosion. We are exploiting both our direct methods approach as well as careful electron microscopy to
understand the atomic scale structures.
- How heteroepitaxy occurs on strontium titanate
Cook, S., K. Letchworth-Weaver, I.C. Tung, T.K. Andersen, H. Hong, L.D. Marks, and D.D. Fong
Sci Adv, 2019. 5(4), eaav0764.
- Electronic structure of lanthanide scandates
Mizzi, C.A., P. Koirala, and L.D. Marks
Physical Review Materials, 2018. 2(2), 025001
- Pauling's rules for oxide surfaces
Andersen, T.K., D.D. Fong, and L.D. Marks
Surface Science Reports, 2018. 73(5), 213-232.
- Transition from Order to Configurational Disorder for Surface Reconstructions on SrTiO3(111)
Marks, L.D., A.N. Chiaramonti, S.U. Rahman, and M.R. Castell
Phys Rev Lett, 2015. 114(22), 226101.
Nanotribology
Friction is a pervasive problem, by some estimates consuming about 5% of the GDP of the economies of the developed world, and a recent analysis has indicated that about one
third of the fuel energy in automobiles goes to overcoming frictional losses. While the importance of minimizing friction can be traced back at least as far as the tomb of Tehuti-Hetep, circa
1880 B.C, where a man can be seen pouring a lubricant to assist in moving a statue, there are still many unknowns in the field of tribology that encompasses friction as well as other critical
processes, such as wear and lubrication. My interests lie in understanding the materials science of sliding at the nanoscale using both in-situ experimentation as well as theory.
- In situ observations of graphitic staples in crumpled graphene
Lin, A.Y.W., X.X. Yu, A. Dato, G. Krauss, and L.D. Marks
Carbon, 2018. 132, 760-765
- In situ single asperity wear at the nanometre scale
Liao, Y. and L.D. Marks
International Materials Reviews, 2017. 62(2), 99-115
- Graphitic Carbon Films Across Systems
Hoffman, E.E. and L.D. Marks
Tribology Letters, 2016. 63(3), 32.
- Soft Interface Fracture Transfer in Nanoscale MoS2
Hoffman, E.E. and L.D. Marks
Tribology Letters, 2016. 64(1), 16.
Nanoparticles: Plasmonics, Catalysis, and Fundamentals
My group has an active program in nanoparticles, ranging from their use in plasmonics and as catalysts to the fundamentals of their growth, thermodynamics and kinetics.
- Shape, thermodynamics and kinetics of nanoparticles
L. D. Marks
Reference Module in Materials Science and Materials Engineering, 2022
- Nanoparticle shape, thermodynamics and kinetics
L.D. Marks and L. Peng
J Phys Condens Matter, 2016. 28(5), 053001.
- Identification of active sites in CO oxidation and water-gas shift over supported Pt catalysts
K. Ding, A. Gulec, A.M. Johnson, N.M. Schweitzer, G.D. Stucky, L.D. Marks and P.C. Stair
Science, 2015.
- Plasmon Length: A Universal Parameter to Describe Size Effects in Gold Nanoparticles
E. Ringe, M.R. Langille, K. Sohn, J. Zhang, J.X. Huang, C.A. Mirkin, R.P. Van Duyne and L.D. Marks
Journal of Physical Chemistry Letters, 2012. 3(11): p. 1479-1483.
Corrosion
If every human vanished tomorrow, in a century or so the majority of our current technology would have vanished, due to corrosion of metals. Indeed, if we were not able to
control corrosion our current civilization would look very different. It is really important to understand what is taking place at the atomic scale, and link this via experiment and theory to
the macroscale.
- New Insights on the Role of Chloride During the Onset of Local Corrosion: TEM, APT, Surface Energy, and Morphological Instability
Yu, X.X., A. Gulec, K.L. Cwalina, J.R. Scully, and L.D. Marks
Corrosion, 2019. 75(6), 616-627.
- Nonequilibrium Solute Capture in Passivating Oxide Films.
Yu, X.X., A. Gulec, Q. Sherman, K.L. Cwalina, J.R. Scully, J.H. Perepezko, P.W. Voorhees, and L.D. Marks
Phys Rev Lett, 2018. 121(14), 145701.
- Competitive Chloride Chemisorption Disrupts Hydrogen Bonding Networks: DFT, Crystallography, Thermodynamics, and Morphological
Consequences
Marks, L.D.
Corrosion, 2018. 74(3), 295-311.
- Early Stage of Oxidation of Mo3Si by In Situ Environmental Transmission Electron Microscopy
Gulec, A., X.X. Yu, M. Taylor, A. Yoon, J.M. Zuo, J.H. Perepezko, and L.D. Marks
Corrosion, 2018. 74(3), 288-294.
Density Functional Theory
My group extensively uses Density Functional Theory (DFT) calculations to understand surface structures. In addition, I have an interest in the development of algorithms
and methodologies to calculate properties faster and more accurately, and do much of the algorithm development and coding myself in my "spare time".
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Predictive Mixing for Density Functional theory (and other Fixed-Point Problems)
L. Marks
J. Chem. Theory Comput. 17 (2021) 5715-5732
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WIEN2k: An APW+lo program for calculating the properties of solids
P. Blaha, K. Schwarz, F. Tran, R. Laskowski, G. K. H. Madsen, and L. D. Marks
J. Chem. Phys. 152 (2020) 074101
- An Augmented Plane Wave + Local Orbitals Program for Calculating Crystal Properties
Blaha, P., K. Schwarz, G.K.H. Madsen, D. Kvasnicka, J. Luitz, R. Laskowsji, F. Tran, and L.D. Marks
2018: Techn. Universitat Wien, Austria.
- Fixed-Point Optimization of Atoms and Density in DFT
L. D. Marks
Journal of Chemical Theory and Computation 9 (2013) 2786.
- Robust mixing for ab initio quantum mechanical calculations
L.D. Marks and D.R. Luke, Physical Review B 78(7): p. 075114-12, 2008
(A gentler preprint)
- Force calculation for orbital-dependent potentials with FP-(L)APW + lo basis sets
F. Tran, J. Kunes, P. Novak, P. Blaha, L.D. Marks, and K. Schwarz
Computer Physics Communications 179: p. 784-790, 2008
Hip Replacements
Prosthetic implantation is one of the most successful treatments for patients with severe arthritis or rheumatism; it is the difference between a wheelchair and a normal
life. As of 2003, more than 200,000 total hip replacement operations were performed annually in the US, and this number is expected to reach 572,000 by 2030. The bearing surfaces of current
artificial hip replacements on the market are usually made out of ultra-high-molecular-weight polyethylene (UHMWPE), cobalt-chromium-molybdenum (CoCrMo) alloys, ceramics (alumina) or
ceramicized metals (e.g. oxygen diffusion-hardened ZrNb alloy). Unfortunately these materials are not perfect, and there are numerous problems. We are investigating the fundamentals of the
metallurgy, tribology, corrosion as well as exploring some of the biological issues, in collaboration with scientists and physicians at Rush Orthopedics and elsewhere.
- The effect of contact load on CoCrMo wear and the formation and retention of tribofilms
M.A. Wimmer, M.P. Laurent, M.T. Mathew, C. Nagelli, Y. Liao, L.D. Marks, J.J. Jacobs and A. Fischer
Wear, 2015. 332–333(0): p. 643-649
- Intergranular pitting corrosion of CoCrMo biomedical implant alloy
Panigrahi, P., Y. Liao, M. Mathew, M.A. Wimmer, J.J. Jacobs, and L.D. Marks
Journal of Biomedical Research, 2013, 102B, 850-859
- CoCrMo metal-on-metal hip replacements.
Y. Liao, E. Hoffman, M.A. Wimmer, A. Fischer, J.J. Jacobs, and L.D. Marks
Physical Chemistry and Chemical Physics. , 15 (2013) 746.
- Graphitic Tribological Layers in Metal-on-Metal Hip Replacements (Supporting
Info)
Y. Liao, R. Pourzal, M. A. Wimmer, J. J. Jacobs, A. Fischer and L. D. Marks
Science 334 (2011) 1687